Antiferromagnetic and Heavy Metal Interfaces

Optimizing Spin-Orbit Torque with Antiferromagnetic and Heavy Metal Interfaces

In the realm of spintronics, optimizing spin-orbit torque (SOT) presents a significant challenge and opportunity. Researchers increasingly explore the interplay between antiferromagnetic materials and heavy metals. By leveraging the unique properties of these materials, we can significantly boost SOT efficiency. Understanding the mechanisms behind these interfaces is essential. In this article, we will explore how antiferromagnetic and heavy metal Interfaces contribute to advance next-generation memory devices.

Introduction to Spin-Orbit Torque

Spin-orbit torque (SOT) plays a crucial role in the field of spintronics, where both the charge and spin of electrons are utilized for data processing and storage. SOT arises from the interaction between the electron’s spin and its orbital motion. This interaction generates a torque on the magnetic moments of materials, enabling efficient manipulation of their magnetization.

In basic terms, when a current flows through a heavy metal with strong spin-orbit coupling, it creates a spin-polarized current. This current results in the generation of a spin accumulation at the interface between the heavy metal and an adjacent magnetic material, such as an antiferromagnet. The key here lies in the relationship between the charge current density (J) and the spin current density ($J_s$), which can be expressed as:

$J_s​$=α⋅J

Here, α represents the spin Hall angle, a measure of how effectively the charge current generates spin polarization.

Once the spin accumulation occurs, it exerts a torque on the magnetic moments. This torque can be quantified using the following equation:

This equation illustrates how the spin current interacts with the magnetization, leading to a change in the magnetic orientation.

SOT offers several advantages over traditional magnetic field-based techniques. First, it requires less power to switch magnetization, enhancing energy efficiency. Second, it enables faster switching times, which is vital for high-speed data processing. As a result, SOT holds immense potential for developing next-generation memory and logic devices.

In summary, understanding spin-orbit torque and its underlying principles is essential for advancing spintronic technology. The ability to manipulate magnetization using spin currents paves the way for innovative applications in data storage and processing.

Landau-Lifshitz-Gilbert equation

The Landau-Lifshitz-Gilbert (LLG) equation is crucial for understanding the dynamics of magnetization in magnetic materials, particularly in the context of spin-orbit torque (SOT)-based memory devices. This equation combines the effects of magnetization precession around an effective magnetic field with damping, providing insights into how magnetization changes over time.

LLG Equation

The LLG equation is expressed as:

Importance of the LLG Equation in SOT-Based Memory Devices

The LLG equation provides a fundamental framework for modeling magnetic dynamics in SOT-based memory devices. By understanding how magnetization responds to external influences—such as SOT generated by spin-polarized currents—researchers can optimize device performance. This optimization enhances the efficiency and speed of writing and reading operations in spintronic memory, paving the way for next-generation data storage technologies.

Fundamental Concepts of Spintronics

Spintronics, short for spin transport electronics, focuses on harnessing the intrinsic spin of electrons, along with their charge, for data storage and processing. Traditional electronics rely only on the charge of electrons to transmit information. Spintronics, however, uses both the charge and spin, offering a new dimension of functionality.

Key Terms in Spintronics

  1. Spin:
    Spin is an intrinsic property of electrons, similar to charge, representing the electron’s angular momentum. It can have two orientations—”up” or “down.” These spin states act like binary data (0s and 1s), making them suitable for information storage.
  2. Magnetic Materials:
    Spintronics relies heavily on magnetic materials, which have regions with aligned magnetic moments, known as domains. Materials like ferromagnets and antiferromagnets serve as fundamental components. Ferromagnets, like iron, have parallel magnetic moments, while antiferromagnets have oppositely aligned magnetic moments.
  3. Torque:
    Torque refers to the force that causes a change in the orientation of a magnetic moment. Spin-orbit torque (SOT), in particular, allows the manipulation of magnetic states through spin-polarized currents. This makes it possible to switch the direction of magnetization in a device.

Combining Charge and Spin Currents

Integrating charge and spin currents forms the core advantage of spintronics. When a charge current flows through a material with strong spin-orbit coupling, it generates a spin current. This spin current carries the angular momentum of electrons without moving their charges. As a result, it can influence the magnetization of a nearby magnetic layer without the need for external magnetic fields.

This combination enables more efficient data storage and processing methods. For instance, spin-polarized currents can write data in magnetic memory cells by switching their magnetization states, achieving faster and more energy-efficient memory devices. Unlike traditional methods, which rely on magnetic fields for switching, spin currents achieve the same result with lower power consumption. This reduces energy loss and heat generation, crucial for scalable memory technologies.

Role of Antiferromagnetic Materials

Antiferromagnetic materials have become a key focus in spintronics, offering unique properties that set them apart from ferromagnetic materials. In antiferromagnets, adjacent atomic magnetic moments align in opposite directions. This alignment results in a net magnetic moment of zero, creating a material with no overall magnetization in its natural state.

Unique Properties of Antiferromagnetic Materials

  1. Fast Dynamics:
    Antiferromagnets exhibit much faster spin dynamics compared to ferromagnets. Their natural resonance frequencies are in the terahertz range, allowing for quicker switching times. This makes them ideal for high-speed spintronic devices.
  2. Stability Against External Fields:
    The internal structure of antiferromagnetic materials offers strong stability against external magnetic fields. Unlike ferromagnets, they do not easily demagnetize or reorient under external field influences. This stability ensures more reliable performance in spintronic applications.
  3. No Net Magnetization:
    Antiferromagnets have zero net magnetization due to the opposing arrangement of their magnetic moments. This absence of a macroscopic magnetic field leads to reduced magnetic interference, which is crucial for densely packed spintronic devices.

Benefits Over Ferromagnetic Materials

  1. Reduced Stray Fields:
    One of the main advantages of antiferromagnets over ferromagnets is the elimination of stray fields. Ferromagnetic materials generate stray magnetic fields due to their non-zero net magnetization. These fields can interfere with neighboring components in integrated circuits, leading to potential data loss or cross-talk. Antiferromagnets, with their zero stray fields, avoid such issues, enabling better scalability of spintronic devices.
  2. Enhanced Data Security:
    Antiferromagnetic materials provide enhanced data security in spintronic applications. Their magnetic states remain more stable and less susceptible to external magnetic noise. This makes them particularly valuable in data storage devices where data integrity is essential.
  3. Compact and Energy-Efficient Design:
    Antiferromagnetic spintronic devices enable more compact designs. Without the need to counteract stray fields, engineers can place components closer together. This feature, combined with their fast dynamics, leads to reduced power consumption and energy-efficient operation, making antiferromagnets suitable for next-generation memory devices..

Measuring Spin in Antiferromagnets

Antiferromagnets offer unique benefits for memory applications, despite not having a net magnetization. Unlike ferromagnets, where the magnetic moments align in the same direction, antiferromagnets have opposing magnetic moments that cancel out. This means no external magnetic field emanates from the material. However, the internal spin structure of antiferromagnets still responds to electrical currents and generates spin currents that can be harnessed for SOT.

Measuring the spin state in antiferromagnets requires specialized techniques since conventional magnetic sensors detect only net magnetization. One common method involves using spin Hall magnetoresistance (SMR). In this technique, an electrical current is passed through a heavy metal adjacent to the antiferromagnet. The interaction between the spin currents from the heavy metal and the spin structure in the antiferromagnet changes the resistance of the heavy metal layer, indirectly revealing information about the spin state.

Another method uses x-ray magnetic linear dichroism (XMLD), where researchers analyze how x-rays are absorbed differently based on the spin orientation in the antiferromagnets. This approach allows high-resolution imaging of the spin order, helping to measure the internal magnetic structure without needing net magnetization.

Heavy Metals and Their Contribution to SOT

Heavy metals play a vital role in generating spin-orbit torque (SOT), making them essential for advanced spintronic devices. These materials exhibit strong spin-orbit coupling due to their high atomic numbers. This coupling creates an interaction between the spin and orbital motion of electrons, which becomes key in converting charge currents into spin currents.

How Heavy Metals Facilitate Spin-Orbit Coupling

Spin-orbit coupling arises naturally in heavy metals. When a charge current flows through these materials, their strong spin-orbit coupling results in the separation of electron spins. This phenomenon gives rise to the spin Hall effect, where a transverse spin current gets generated perpendicular to the charge current. The spin current then accumulates at the interface between the heavy metal and a magnetic layer.

This spin accumulation creates an effective magnetic field that exerts torque on the magnetization of the adjacent magnetic layer. As a result, the spin-polarized current can manipulate the magnetic state without relying on external magnetic fields. This mechanism is what makes heavy metals so effective for SOT-based memory and logic devices.

Commonly Used Heavy Metals in SOT Research

  1. Platinum (Pt):
    Platinum has become a popular choice in SOT research due to its strong spin-orbit coupling and high spin Hall angle. Researchers value Pt for its efficiency in generating spin currents, making it ideal for switching magnetic layers. Additionally, its stability and compatibility with various magnetic materials ensure robust performance in spintronic applications.
  2. Tungsten (W):
    Tungsten exhibits a high spin Hall angle, even higher than platinum, which allows for stronger spin-current generation. Researchers often use tungsten in SOT studies where greater efficiency is required. However, it is crucial to control the crystalline phase of tungsten, as its properties can vary significantly between phases like α\alphaα-W (less spin-orbit coupling) and β\betaβ-W (more spin-orbit coupling). Proper phase management enables researchers to maximize its SOT performance.
  3. Tantalum (Ta):
    Tantalum has also gained attention for SOT studies. It can exist in two phases, α\alphaα and β\betaβ, with β\betaβ-Ta being particularly effective for spin current generation due to its high spin Hall angle. Tantalum’s unique properties make it a valuable material for experiments aiming to optimize SOT efficiency in memory devices.

Contributions of Heavy Metals to Efficient SOT

Heavy metals like platinum, tungsten, and tantalum enable efficient control over magnetization through spin-orbit torque. They convert charge currents into spin currents, allowing for lower power switching of magnetic states. This property not only improves energy efficiency but also enables faster data writing speeds, crucial for next-generation memory devices. By selecting the right heavy metal, researchers can tailor SOT behavior to suit specific applications, pushing the boundaries of what spintronics can achieve.

Overall, the use of heavy metals with strong spin-orbit coupling is a cornerstone of SOT-based spintronic devices. Their ability to generate effective spin currents drives advancements in energy-efficient, high-speed memory technologies.

Interface Engineering

Optimizing the interfaces between antiferromagnetic and heavy metal layers plays a critical role in enhancing spin-orbit torque (SOT) performance. These interfaces directly influence the strength of spin currents and the efficiency of spin transfer, making them key to achieving high-performance spintronic devices.

Importance of Interface Optimization

  1. Spin Transparency:
    A well-engineered interface ensures efficient transfer of spin currents from the heavy metal into the adjacent antiferromagnetic layer. The goal is to maximize spin transparency—the ability of the interface to transmit spin information with minimal loss. Higher spin transparency allows for stronger spin currents, which, in turn, produces a more effective SOT.
  2. Reducing Spin Memory Loss:
    Imperfections at the interface, such as roughness or intermixing of layers, can lead to spin scattering and spin memory loss. This reduces the spin current that reaches the antiferromagnetic layer, decreasing the torque exerted on its magnetization. Proper interface engineering minimizes these imperfections, ensuring that more spin angular momentum reaches the target layer.
  3. Interfacial Spin-Orbit Coupling:
    The interface between a heavy metal and an antiferromagnetic material can modify the spin-orbit coupling properties, influencing how the spin currents behave. Adjusting the chemical composition or crystalline structure at the interface can amplify the spin Hall effect, resulting in a more efficient generation of spin currents.

Impact of Interfacial Properties on SOT Efficiency

  1. Spin Current Generation:
    The properties of the interface determine how effectively a charge current in the heavy metal converts into a spin current. Materials with high spin-orbit coupling, like platinum or tungsten, generate robust spin currents, but the interface needs to facilitate their transfer. A smoother and well-defined interface boosts this process, leading to better SOT efficiency.
  2. Switching Threshold:
    The interfacial quality also affects the switching threshold—the minimum current needed to change the magnetic state in the antiferromagnetic layer. A well-optimized interface reduces this threshold, enabling lower power operation. This makes the device more energy-efficient and extends its lifetime.
  3. Thermal Stability:
    The thermal stability of the interface impacts the long-term reliability of spintronic devices. During device operation, temperature variations can cause changes in interfacial properties. Engineers focus on developing robust interfaces that maintain spin transparency and coupling even under thermal stress, ensuring consistent performance.

Overall Device Performance

By focusing on interface engineering, researchers can significantly enhance SOT-based device performance. Optimized interfaces allow for stronger spin torques, lower power requirements, and faster switching speeds. This makes SOT-based memory devices more competitive with traditional technologies, offering a pathway to more efficient, reliable, and scalable memory solutions. Ultimately, the quality of the interface can make or break the performance of spintronic devices, highlighting its importance in next-generation technology.

Experimental Techniques

Studying and characterizing spin-orbit torque (SOT) requires precise experimental techniques. These methods help researchers understand the behavior of spin currents, magnetic switching, and the structural properties of the materials involved. Key techniques include magnetotransport measurements and x-ray diffraction, among others. Recent advancements have further refined these tools, enabling more accurate and detailed analysis.

Key Techniques for SOT Characterization

  1. Magnetotransport Measurements:
    Magnetotransport measurements analyze how electrical resistance changes in response to an applied magnetic field. Techniques like the Hall effect and anomalous Hall effect (AHE) provide insight into the behavior of spin currents in heavy metals and their influence on adjacent magnetic layers. These measurements help quantify the efficiency of spin-orbit torque and reveal the switching characteristics of spintronic devices. Using second harmonic Hall measurements, researchers can directly evaluate the strength of spin-orbit coupling and the damping-like torque generated by spin currents.
  2. X-Ray Diffraction (XRD):
    X-ray diffraction offers a powerful way to study the structural properties of thin films and heterostructures. Researchers use XRD to determine the crystalline quality, phase composition, and strain in both heavy metal and antiferromagnetic layers. High-quality crystallinity enhances spin current flow and spin-orbit torque efficiency. XRD data helps refine growth techniques and optimize film quality for improved device performance.
  3. Spin-Torque Ferromagnetic Resonance (ST-FMR):
    ST-FMR measures the dynamics of magnetization under the influence of microwave currents. Researchers use this technique to extract parameters like spin Hall angle and damping constant, which directly relate to the efficiency of SOT. ST-FMR helps to identify how spin currents impact the magnetic layer’s precession, giving a detailed view of spin dynamics at the interface.
  4. Brillouin Light Scattering (BLS):
    Brillouin light scattering is a non-invasive optical technique that probes spin waves in magnetic materials. BLS detects the scattering of light by spin waves, allowing researchers to study spin interactions at the interface between antiferromagnetic and heavy metal layers. This technique provides detailed information about the exchange interactions and spin dynamics, crucial for understanding how to optimize spin-orbit torques.

Recent Advancements in Measurement Techniques

  1. Time-Resolved Magneto-Optical Kerr Effect (TR-MOKE):
    TR-MOKE has become a valuable tool for studying ultrafast spin dynamics in SOT systems. This technique tracks changes in magnetization on femtosecond timescales using laser pulses. It enables the observation of spin switching and domain wall motion in real-time, providing insights into the speed and efficiency of SOT-based switching mechanisms.
  2. X-Ray Magnetic Circular Dichroism (XMCD):
    XMCD, performed at synchrotron facilities, allows element-specific probing of magnetic properties at interfaces. It provides a deeper understanding of how individual atomic layers in complex heterostructures contribute to SOT. This technique has become crucial for characterizing interfacial spin-orbit coupling effects with high spatial resolution.
  3. Scanning Transmission Electron Microscopy (STEM) with Electron Energy Loss Spectroscopy (EELS):
    Researchers use STEM-EELS to study the atomic structure and composition at interfaces with sub-nanometer resolution. This helps reveal how interfacial roughness or atomic intermixing influences SOT performance. STEM-EELS has proven valuable in developing high-quality interfaces that maximize spin current transmission.

These advanced techniques allow researchers to unravel the complexities of spin-orbit torque and its impact on device performance. Combining them provides a more comprehensive understanding of both spin dynamics and structural properties. As these methods continue to evolve, they drive progress in the development of more efficient, reliable SOT-based memory and logic devices.

Recent Research and Developments

Recent studies have made significant progress in optimizing spin-orbit torque (SOT) for spintronic devices. Researchers continue to explore new materials, innovative synthesis methods, and advanced characterization techniques. These advancements aim to enhance the efficiency of spin current generation and improve the stability of antiferromagnetic/heavy metal interfaces.

Notable Studies in SOT Optimization

  1. Exploring New Heavy Metal Materials:
    A study published in Nature Electronics investigated the use of novel heavy metal alloys to improve spin current efficiency. Researchers combined materials like platinum-iridium alloys to enhance spin-orbit coupling while reducing resistivity. These alloys demonstrated improved SOT generation, resulting in lower switching currents and faster response times. This study provided a pathway to developing more energy-efficient spintronic memory devices.
  2. Integration of 2D Materials with SOT Systems:
    Another breakthrough involved using two-dimensional (2D) materials like graphene and transition metal dichalcogenides (TMDs) in SOT devices. Researchers observed that stacking these 2D materials with traditional heavy metals can enhance spin injection efficiency and reduce charge-current-induced heating. This integration not only increases SOT efficiency but also opens the door to scalable, flexible spintronic applications.
  3. Engineering Phase-Controlled Tantalum (Ta):
    A recent study focused on controlling the crystalline phase of tantalum to enhance SOT. By adjusting deposition parameters, researchers optimized the growth of β-Ta over α-Ta. This phase offers a higher spin Hall angle, boosting spin current conversion. Improved deposition techniques allowed for the stable growth of β-Ta, leading to better control over SOT efficiency. This advancement emphasized the importance of tailoring material phases for spintronic performance.

Innovative Approaches in Synthesis and Characterization

  1. Atomic Layer Deposition (ALD) for Precise Interface Control:
    Atomic layer deposition (ALD) has emerged as a precise method for synthesizing antiferromagnetic/heavy metal heterostructures. ALD allows for atomic-level control over film thickness and uniformity, which is crucial for achieving high-quality interfaces. Studies have shown that ALD can create smoother interfaces with fewer defects, enhancing the spin transparency and overall SOT performance. This approach ensures better consistency and reproducibility in device fabrication.
  2. Magnetic Proximity Effects in SOT Devices:
    Recent research has focused on magnetic proximity effects to fine-tune interfacial properties. By introducing ultrathin ferromagnetic layers at the interface between a heavy metal and antiferromagnetic material, researchers can manipulate the interfacial spin orientation. This method creates a more effective spin injection layer, leading to stronger SOT-induced switching. It also provides a means to control the interfacial exchange coupling, improving the robustness of the magnetic states.
  3. Advanced X-Ray Imaging Techniques:
    Studies have also utilized advanced X-ray imaging methods like X-ray photoemission electron microscopy (XPEEM) to visualize spin textures at interfaces. XPEEM provides high-resolution images of the magnetic states, revealing how spin structures evolve during SOT switching. These insights help researchers understand the role of interfacial spin interactions and refine synthesis methods to achieve optimal spin-orbit torque performance.
  4. Room-Temperature SOT in Antiferromagnetic Insulators:
    A groundbreaking study demonstrated room-temperature SOT in antiferromagnetic insulators like NiO paired with platinum. Researchers showed that spin currents could efficiently transfer from Pt into NiO, achieving robust control over the antiferromagnetic order. This finding indicates the potential for using insulating antiferromagnets in low-power, high-speed spintronic applications, marking a significant shift from conventional metallic systems.

These recent studies have deepened the understanding of SOT mechanisms and have provided innovative approaches to interface engineering. By optimizing material selection, deposition techniques, and characterization methods, researchers push the boundaries of what SOT-based devices can achieve. These advancements bring the field closer to realizing practical, energy-efficient spintronic memory and logic solutions.

Applications in Spintronics-Based Devices

Optimized spin-orbit torque (SOT) opens up exciting possibilities for next-generation spintronic devices. Its ability to efficiently manipulate magnetization using electrical currents makes it ideal for memory storage and logic applications. As the technology advances, SOT-based devices promise faster speeds, lower power consumption, and greater durability compared to conventional semiconductor technologies.

Memory Devices

  1. SOT-MRAM (Magnetoresistive Random-Access Memory):
    SOT-MRAM stands out as one of the most promising applications. Unlike traditional MRAM, SOT-MRAM uses spin currents to switch magnetic states without needing a high current through the memory cell. This enables faster write speeds and reduces energy consumption. SOT-MRAM also offers non-volatility, ensuring data retention even without power. With these advantages, SOT-MRAM can replace existing non-volatile memory technologies, like Flash, in various computing systems.
  2. Cache Memory in CPUs:
    SOT-MRAM can serve as cache memory in high-performance CPUs. It delivers low latency, enabling faster data access for processing tasks. As the demand for quicker and more efficient computing increases, SOT-MRAM can improve the performance of CPUs in data centers, AI systems, and mobile devices.
  3. Neuromorphic Computing:
    Researchers explore SOT-based devices for neuromorphic computing, which aims to mimic the brain’s neural networks. SOT’s fast switching capabilities can enable synapse-like behavior in artificial neurons. This makes it a strong candidate for building efficient, brain-inspired processors, capable of tackling complex AI tasks.

Logic Applications

  1. Reconfigurable Logic Gates:
    SOT enables the creation of reconfigurable logic gates, where a single device can switch between different logical operations. This reduces the number of transistors required, saving space and power. Reconfigurable gates also allow more flexibility in designing compact and efficient processors.
  2. Spintronic Logic Circuits:
    Spintronic circuits, using SOT, can process information with high-speed magnetic domain wall motion. These circuits promise faster processing while consuming less power than traditional silicon-based logic circuits. They can be especially beneficial in applications requiring fast data processing, such as edge computing and real-time data analysis.

The Future of Spintronic Devices

SOT-based devices hold potential to transform the electronics industry. As fabrication techniques improve, they could become integral components of mainstream memory and logic devices. Their inherent speed, scalability, and energy efficiency align well with the needs of future technologies, including AI, IoT, and edge computing. Moreover, their ability to operate in harsh environments and withstand radiation makes them ideal for space and defense applications.

Challenges and Future Directions

Despite their promise, several challenges remain in optimizing spin-orbit torque for practical applications. Overcoming these obstacles will determine the success of SOT in future devices.

Current Challenges

  1. Material Compatibility:
    Finding the right combination of antiferromagnetic and heavy metal layers poses a significant challenge. Researchers aim to identify materials that offer high spin-orbit coupling, thermal stability, and easy integration with current semiconductor processes. Balancing these factors can be difficult, as not all materials exhibit consistent performance.
  2. Interface Stability:
    Achieving stable interfaces between materials is crucial for reliable SOT performance. Interface roughness, atomic intermixing, and defects can lead to reduced spin transparency, affecting efficiency. Long-term stability under operating conditions, including temperature variations, remains a hurdle that must be addressed to ensure device longevity.
  3. Power Consumption and Scalability:
    While SOT reduces switching energy compared to traditional methods, achieving ultra-low power consumption in scalable devices remains a goal. Researchers focus on minimizing the current required for switching without sacrificing speed. Scaling down the size of SOT devices to match the requirements of modern nanotechnology also requires precise control over fabrication processes.

Future Research Directions

  1. Novel Material Exploration:
    The search for new materials with high spin Hall angles and strong spin-orbit coupling continues. Alloys, heterostructures, and 2D materials offer potential improvements. Integrating these into existing SOT devices could lead to significant efficiency gains.
  2. Hybrid Spintronic Devices:
    Researchers explore hybrid spintronic devices that combine SOT with other effects, like spin-transfer torque (STT) or magnetoelectric effects. This hybrid approach could lower power consumption further and enable multifunctional devices that blend memory and logic functions into a single unit.
  3. Room-Temperature Operation:
    Expanding the temperature range at which SOT operates efficiently remains a priority. Achieving stable room-temperature operation in antiferromagnetic materials could bring SOT-based devices closer to practical deployment in commercial electronics.
  4. Advanced Fabrication Techniques:
    Developing new deposition methods, like molecular beam epitaxy (MBE) and atomic layer deposition (ALD), will enhance control over film quality and interfaces. This will help researchers tailor material properties and create high-quality heterostructures, improving SOT efficiency.

The path toward optimizing SOT for real-world applications involves overcoming material challenges and refining fabrication techniques. As research advances, the future of spintronics-based devices looks promising. These devices could redefine memory and logic technologies, paving the way for faster, more energy-efficient electronics. With continued progress, SOT-based technologies hold the potential to shape the next wave of innovation in computing and data storage.

End Note

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